Sequential multiphoton excitation method

摘要

Efficient multiphoton excitation is accomplished by sequentially exciting a polyatomic molecule with one or more wavelengths of infrared laser radiation. Preferably, the delay between successive excitations is longer than the rotational but shorter than the vibrational relaxation time of the molecule. By this method, laser-induced chemical reactions or isotope separation can be achieved with lower fluence and/or higher concentration of molecules than with prior art methods.